Twice, once in the NL in 1961 and again in the AL in 1966.
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Frank Robinson won the NL MVP in 1961 when he played for Cincnnati and won the AL MVP in 1966 when he was with Baltimore.
Frank Robinson. Frank Robinson won the 1961 NL MVP as a member of the Cincinnati Reds and, the 1966 AL MVP as a member of the Baltimore Orioles.
Frank Robinson was a Major League Baseball outfielder and manager. He is the only player to win MVP honors in both the National and American Leagues. He has won the triple crown, World Series (2X) and was elected to the baseball hall of fame in 1982.
Frank Robinson was National League Rookie of the Year in 1956, American League Triple Crown winner in 1966, National League MVP in 1961 and American League MVP in 1966. I don't know of a second.
Elgin Baylor was never named NBA MVP.