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1966
Twice, once in the NL in 1961 and again in the AL in 1966.
5-3 games where won when jackie was in the dodgers
Frank Robinson won the NL MVP in 1961 when he played for Cincnnati and won the AL MVP in 1966 when he was with Baltimore.
No, only once -- in 1966. He did, however, win two MVPs -- the only person to do so in both leagues.