In the entire history of MLB, that is the Giants.
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Considering that the Yankees have 26 world titles and have been to at least 6 more I would see the New York Yankees.
The New York Yankes won 26 World Series titles in 39 appearances.
Through the 2010 season, that is the Houston Astros with 9 playoff appearances without a World Series win.
The New York Yankees have played in the most World Series games.
The New York Yankees appeared in 40 World Series, and won 27.
As of 2011, the New York Yankees have won the most World Series, capturing the trophy 27 times.