As far as the Cardinals' best season in Arizona, it would have to be 1998. After posting a 9-7 regular season record & qualifying for the postseason via wild card, they traveled to Dallas and defeated the Cowboys, 20-7. This playoff win was the first for the franchise since 1947, when the then-Chicago Cardinals won the NFL championship.
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2002.
The NFC realigned from 3 five team divisions to 4 four team divisions in 2002. The Falcons, Saints, and Panthers Left the NFC West for the newly formed NFC South division, the Cardinals moved from the NFC East to the NFC West, and the Seattle Seahawks moved from the AFC West to the NFC West. The 49ers and Rams stayed in the NFC West.